Foods rich in magnesium can help relax the muscles, and things like a tea of of herbal and natural remedies that can help alleviate muscle spasms, and the. Mar 26, Furthermore, valerian root is one of the top herbs to use when you need pain relief combined with muscle relaxation. In addition, studies. Chamomile is an ancient herb that's used to treat a variety of ailments, including Another sweet and natural way to relax your muscles is by eating blueberries. Natural Muscle Relaxation Teas for Anyone Suffering From Muscle Spasms or Other Muscular Ailments Feb 21, Herbal muscle relaxers are basically types of special natural herbs that have the ability to cause body muscles to relax. Thus alleviating pain. Sep 21, Common natural muscle relaxants are chamomile and valerian. These two herbs relax the muscles. They are often used in aromatherapy. Feb 20, Magnesium is a mineral that's required for muscle relaxation (2). . Valerian root is a medicinal herb often used as a natural muscle relaxer.